Resonance-enhanced x-ray multiple ionization of a polyatomic molecule

نویسندگان

چکیده

Extremely high charge states of atoms and molecules can be created when they are irradiated by intense x-ray pulses. At certain photon energies, electron ejection from drastically enhanced transient resonances during the sequential ionization process. Here we report on observation such resonance effects in a molecule, CH3I, show photon-energy-dependent shift resonance-induced structures ion state distributions. By comparing distribution CH3I with that atomic xenon, molecule-specific features observed, which attributed to ultrafast intramolecular rearrangement. In addition, experimentally demonstrate charge-rearrangement-enhanced molecules, previously found hard x rays, also plays role soft regime.Received 5 February 2022Revised 9 March 2022Accepted 15 April 2022DOI:https://doi.org/10.1103/PhysRevA.105.053102©2022 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasAtomic & molecular processes external fieldsAutoionization Auger processesElectronic excitation ionizationUltrafast phenomenaAtomic, Molecular Optical

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ژورنال

عنوان ژورنال: Physical Review A

سال: 2022

ISSN: ['1538-4446', '1050-2947', '1094-1622']

DOI: https://doi.org/10.1103/physreva.105.053102